Modern Aspects of Diffusion-Controlled Reactions: Cooperative Phenomena in Bimolecular Processes - Image 1

£315.00

Elsevier Modern Aspects of Diffusion-Controlled Reactions: Cooperative Phenomena in Bimolecular Processes

Name: Modern Aspects of Diffusion-Controlled Reactions: Cooperative Phenomena in Bimolecular Processes
Brand: Elsevier
Price: 315.0 GBP
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Physical Chemistry

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Description

This monograph deals with the effects of reactant spatial correlations arising in the course of basic bimolecular reactions describing defect recombination, energy transfer and exciton annihilation in condensed matter. These effects lead to the kinetics considered abnormal from the standard chemical kinetics point of view. Numerous bimolecular reaction regimes and conditions are analysed in detail. Special attention is paid to the development and numerous applications of a novel, many-point density (MPD) formalism, which is based on Kirkwood's superposition approximation used for decoupling three-particle correlation functions. The book demonstrates that incorporation of the reaction-induced spatial correlations of similar reactants (e.g, vacancy-vacancy) leads to the development of an essentially non-Poisson spectrum of reactant density fluctuations. This can completely change the kinetics at longer times since it no longer obeys the law of mass action. The language of the correlation lengths and critical exponents similar to physics of critical phenomena is used instead. A relation between MPD theory and synergistics is discussed. The validity of the theorem giving a critical complexity for the two-step reactions exhibiting self-organization phenomena is questioned. Theoretical results are illustrated by numerous experimental data.

Product Specifications

Brand: Elsevier
Format: paperback
ASIN: 0444543910
Category: Books > Subjects > Science, Nature & Maths > Chemistry > Physical Chemistry
Domain: Amazon UK
Release Date: 06 August 2011
Listed Since: 11 July 2011

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Elsevier Modern Aspects of Diffusion-Controlled Reactions: Cooperative Phenomena in Bimolecular Processes

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